I don't think I'm educated enough to know that one. Magazines write about cornering Gs just over 1.0 on street tires, so I would have guessed that braking (or cornering) with racier tires would be higher Gs. If you have an accelerometer, how high are cornering Gs?
I'm going to guess again and say braking could produce higher Gs than cornering because in a corner, the rear wheels are also asked to push as well. Therefore they can't devote all effort to one direction, which in braking they could.
But then again, wheel alignment under cornering is designed for best cornering. Under extreme braking you might produce toe out and more camber, which may limit braking... (I don't think people get an alignment for best braking.)
The obvious dumb answer to how much brake to add - can you lock them up now? If yes, then you have enough brake and need more tire.
If you have the equipment to try again, leave the clutch engaged. Asking the rear brakes to also decelerate the engine will lessen their impact on decelerating the car weight and you can perhaps judge whether the rears are locking or not.
Lime Rock Park in Connecticut has a 140MPH to 70MPH (I think 70, but I am never looking) and under braking my car dances. As each tire rises and falls over the uneven pavement it gets more and less grip. It's very interesting how it affects the yaw of the car - happens quickly enough I can't really keep up with it, but happens sufficiently to each wheel that on average the car stays straight.
Iridium on this board has experience with Toyos, Vipers, 40mm rears, and an accelerometer. We'll have to page him, too.